Safety first - do not mess with compressed air if you do not fully understand.
BAR and PSI are very different things.
http://www.centauro-owners.com/articles/psibar.html
Size equates to capacity not pressure. Note the bigger the cylinder the more air it will hold, not the higher the pressure.
When using a large cylinder to fill paintball cylinders the pressure will still drop, so if filling from empty you need to fill the individual cylinders to a lower pressure to extend the time it takes the master cylinder to drop in pressure, or keep topping up from a compresor.
You will need a high pressure compressor not a tyre compressor or air brush compressor, but it must also be clean air.
These cost thousands, but a cheaper compressor had been announced in the US.
It is most likely not worth it - go to paintball sies or dive shops for cylinder fills.
Or if you have a non electric marker you can tweak with disposable CO2 and an adaptor.
Air left at the end of the day is usually sufficient for any home tweaking. (Technically you should not be transporting compresed air - have you told the insurers of any vehicles you travel from sites?) We may or may not need to legally have to display the compressed air sign as a private traveller - but the fire brigade would certainly prefer it is displayed even if you only have a half full 3000psi steel cylinder. They won't be impressed if they are cuttng you out of your car crash and find a cylinder.
If you have a genuine need for a private fill rig then get a scuba rig AND THE INSTRUCTION TO USE IT SAFELY.